Method for metathesis of compounds comprising an olefinic...

Chemistry of hydrocarbon compounds – Unsaturated compound synthesis – By alkyl transfer – e.g. – disproportionation – etc.

Reexamination Certificate

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C585S643000

Reexamination Certificate

active

07635794

ABSTRACT:
The invention relates to a method for metathesis of one or several reagents comprising a linear or branched hydrocarbon chain containing a double olefinic bond Csp2═Csp2consisting in reacting said reagent or reagents with a supported metal compound comprising an aluminum oxide-based support to which a tungsten hydride is grafted. Typically, each said reagent or reagents comprises from 2 to 30 carbon atoms. The reagent can be embodied in the form of olefin. The inventive method can be used, for example for producing propylene from ethylene and butane.

REFERENCES:
patent: 3634538 (1972-01-01), Steffgen
patent: 3865751 (1975-02-01), Banks et al.
patent: 6229060 (2001-05-01), Vidal et al.
patent: 6632765 (2003-10-01), Chen
patent: 2002/0002317 (2002-01-01), Schwab et al.
Levisalles et al, “Etudes sur le mecanisme de la metathese des olefins i”, 1980, pp. 195-207, vol. 192, No. 2, J. Organometallic Chemistry, The Netherlands.
Wengrovius et al, “Multiple metal-carbon bonds. 25. Preparation and structure of tungsten neopentylidene hydride, neopentylidene carbonyl, and neopentylidene ethylene complexes”, 1982, p. 1739-1740, vol. 104, No. 6, Journal of the American Chemical Society.

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