Method for desulfurizing a gas

Chemistry of inorganic compounds – Modifying or removing component of normally gaseous mixture – Sulfur or sulfur containing component

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Details

42324409, 423220, 423222, 4235742, 423575, 423230, C01B 1704, C01B 1716

Patent

active

053893514

ABSTRACT:
A foul gas containing H.sub.2 S is brought into the presence of SO.sub.2 in a first stage to permit the reaction between SO.sub.2 and H.sub.2 S to form water and elemental sulfur. The SO.sub.2 is solubilized in an absorbent composition which includes a solvent for both SO.sub.2 and H.sub.2 S so that the H.sub.2 S in the foul gas is first solubilized in the absorbent composition where it is then brought into contact with the solubilized SO.sub.2 for reaction between a major portion of the H.sub.2 S and the solubilized SO.sub.2 to form elemental sulfur. The gas is then passed to a second stage where any remaining H.sub.2 S is removed by aqueous catalytic reaction of the type conventional in the prior art. The apparatus utilized to carry out the present invention preferably includes a two stage column in which the first stage provides the absorbent material containing solubilized SO.sub.2 for reaction with the H.sub.2 S of the foul gas. During the SO.sub.2 extraction stage the major portion of the H.sub.2 S is removed from the foul gas. The gas is then conveyed from the first stage to a second stage which comprises a conventional aqueous catalytic scrubbing operation where the remainder of the H.sub.2 S is removed. The absorbent composition utilized in the process comprises solvents that dissolve SO.sub.2 and/or H.sub.2 S which can be heated to a temperature above the melting point of sulfur without detrimentally affecting the solvent so that it may be recycled through the system.

REFERENCES:
patent: 3598529 (1971-08-01), Deschamps
patent: 3649190 (1972-03-01), Deschamps
patent: 3880986 (1975-04-01), Beavon
patent: 3937795 (1976-02-01), Hasebe
patent: 3947559 (1976-03-01), Gibson et al.
patent: 4442083 (1984-04-01), Canales et al.
patent: 4976935 (1990-12-01), Lynn
patent: 5120517 (1992-06-01), Elshout

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