Method and apparatus for obtaining pure-absorption two-dimension

Electricity: measuring and testing – Particle precession resonance – Using a nuclear resonance spectrometer system

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324307, G01R 3320

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052627233

ABSTRACT:
A signal function S(t.sub.1, t.sub.2) is obtained from a plurality of coherence transfer pathways in a single acquisition by preparing a molecular system in a coherent non-equilibrium state, and alternately and sequentially detecting signals at individual sampling points, in t.sub.2, from the plurality of coherence transfer pathways by using gradient refocusing of a new pathway after signal detection at a sampling point in another pathway. A frequency domain spectrum S(.omega..sub.1,.omega..sub.2) is constructed by first Fourier transforming the time domain signals S(t.sub.1, t.sub.2) in the t.sub.2 dimension and producing real and imaginary components which modulate as sine and cosine signals in t.sub.1. The real (.omega..sub.2) cosine (t.sub.1) components are combined with the imaginary (.omega..sub.2) sine (t.sub.1) components to form a complex data set S(t.sub.1, .omega..sub.2) that is amplitude modulated in t.sub.1. The complex data set is then Fourier transformed in the t.sub.1 dimension to construct in frequency domain spectrum S(.omega..sub.1, .omega..sub.2) which contains pure absorption lineshapes.

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