Manufacturing process for the preparation of...

Organic compounds -- part of the class 532-570 series – Organic compounds – Carboxylic acids and salts thereof

Reexamination Certificate

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C560S232000, C549S513000

Reexamination Certificate

active

07151192

ABSTRACT:
A manufacturing process for the preparation of α,α-branched alkane carboxylic acids, by reacting a mono-olefin or a precursor thereof, with carbon monoxide in the presence of a strong acid catalyst characterized in that the starting olefin is a dimmer C8 or trimer C12 derived from n-butene, which predominantly comprise 2-butene, that the acid catalyst is composed of BF3/H3PO4in a molar ratio of BF3:H3PO4in the range of from 0.5:1.0 to 5.0:1.0, or of CF3SO3H, that the weight ratio of the catalyst relative to the mono-olefin is in the range of from 1:1 to 10:1, that the reaction is carried out at a temperature in the range of from 60 to 140° C., and with an initial water content in the catalyst system in the range of from 8 to 25 wt %; and vinyl esters and glycidyl esters derived from said carboxylic acids.

REFERENCES:
patent: 2967873 (1961-01-01), Koch et al.
patent: 5229461 (1993-07-01), Saitoh et al.
patent: 5430179 (1995-07-01), Lincoln et al.
patent: 6211406 (2001-04-01), Lange et al.
patent: 6281372 (2001-08-01), Wiese et al.
patent: 6433242 (2002-08-01), Wiese
patent: 972291 (1959-07-01), None
Toho Chemical Industry Co., Ltd., 1983, CAS: 98: 139012.

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