Lithium ion cells with improved thermal stability

Chemistry: electrical current producing apparatus – product – and – Current producing cell – elements – subcombinations and... – Electrode

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429212, H01M 462

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active

060776242

ABSTRACT:
The methods and compositions of the invention provide two solutions to reduce the reactivity of VDF-based copolymers to lithiated graphite. The two approaches can be used separately or combined. In one embodiment, the relative proportion of the VdF and the other fluorinated monomer (OFM, i.e. HFP) in the copolymer is significantly reduced below conventional formulations in order to reduce the reactivity of the copolymer. In a second approach, the reactivity of the copolymer, over a broad range of monomer VdF:OFM molar ratios, is reduced by deactivating the reactive sites on the copolymer, thereby blocking the ability to undergo undesired reaction during cell operation. These methods and compositions have heretofore not been proposed and are of primary importance in preventing large exothermic reaction which can lead to thermal runaway when conventional polymer formulations are utilized in batteries in the presence of reactive components such as lithiated graphite.

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