Isomerization of vinyl glycols to unsaturated diols

Organic compounds -- part of the class 532-570 series – Organic compounds – Oxygen containing

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502 60, C07C 33025, C07C 3303, C07C 3120

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active

058116010

ABSTRACT:
This invention relates to a process for the isomerization of a vinyl glycol to an unsaturated diol in the presence of a rhenium-based catalyst; and to a catalyst for said isomerization. More specifically, this invention relates to the isomerization of 3-butene-1,2-diol to 2-butene-1,4-diol; and to a process for the manufacture of 1,4-butanediol involving the step of isomerizing 3-butene-1,2-diol to 2-butene-1,4-diol in the presence of said catalyst. The catalyst is characterized in that it comprises a transition metal on a carrier wherein the carrier is a zeolite Y type substance containing silicon and aluminum in a mole ratio of from about 1.5:1 to about 1000:1, and the transition metal is rhenium or a rhenium compound and mixtures thereof present in an amount of from about 0.1 to about 50 weight percent based on total combined weight of the carrier and of the rhenium or rhenium compound and mixtures thereof.

REFERENCES:
patent: 2911445 (1959-11-01), Friederich
patent: 5117012 (1992-05-01), Stavinoha, Jr. et al.
patent: 5166372 (1992-11-01), Crocco et al.
patent: 5336815 (1994-08-01), Becker
WPAT abstract of J59 084 831;, 1984.
WPAT abstract of JP 54-073710, 1979.
WPAT abstract of JP 53-127405, 1978.
WPAT abract of 62-054788, 1987.
WPAT abstract of DE 7743846, 1979.
WPAT abstract of JP 49-049910, 1974.

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