Ion exchange enrichment of uranium isotopes

Chemistry of inorganic compounds – Treating mixture to obtain metal containing compound – Radioactive metal

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423 6, C01G 4300

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active

043681751

ABSTRACT:
A process for the enrichment of one isotope in a mixture of uranium isotopes by passing a solution of the mixture in a solvent through an anion exchanger thereby forming on the anion exchanger a boundary (A) between a uranium adsorption zone and an adjacent reducing agent zone and/or a boundary (B) between a uranium adsorption zone and an adjacent oxidizing agent zone, the uranium adsorption zone advancing through the anion exchanger, effecting reduction at the boundary (A) and/or effecting oxidation at the boundary (B), thereby effecting enrichment adjacent said boundary, and separating a fraction enriched in one of said isotopes, which process comprises using as the solvent medium a composition comprising (a) a solvent having a dielectric constant of at least 80 at 20.degree. C., (b) hydrochloric acid and (c) at least one of hydrobromic acid and sulfuric acid, the solvent medium having a hydrogen ion concentration of about 0.1 M/l to about 10 M/l, a total chlorine ion concentration of about 0.1 M/l to about 12 M/l, at least one of bromine and sulfate ion being present in about 0.01 M/l to about 10 M/l and the other being present in from zero up to 10 M/l, and passing the materials through the ion exchanger at a rate such that the migration velocity of the uranium adsorption zone through the ion exchanger is at least about 1 cm per minute.

REFERENCES:
patent: 3953568 (1976-04-01), Seko et al.
patent: 3953569 (1976-04-01), Seko et al.
patent: 4049769 (1977-09-01), Seko et al.
patent: 4112044 (1978-09-01), Miyake et al.
patent: 4112045 (1978-09-01), Seko et al.
patent: 4202860 (1980-05-01), Miyake et al.

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