Insertion compounds based on manganese oxide usable as the posit

Chemistry of inorganic compounds – Oxygen or compound thereof – Metal containing

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429224, C01G 4512

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active

057004420

ABSTRACT:
The invention relates to the preparation of insertion compounds based on manganese oxide, usable as the positive electrode active material in a lithium battery.
These compounds in the hatched area of FIG. 1 can be prepared by reacting in the solid state a manganese oxide powder MnO.sub.2 -.beta., having a specific surface below 7 m.sup.2 /g and an average grain size below 10 .mu.m, with a powder of a lithium compound such as Li.sub.2 CO.sub.3 or LiOH, at a temperature of 150.degree. to 500.degree. C. for an adequate time to convert the .beta.-MnO.sub.2 into manganese and lithium oxide having a lacunary or stoichiometric spinel structure.

REFERENCES:
patent: 4959282 (1990-09-01), Dahn et al.
Journal of the Electrochemical Society, vol. 141, No. 1, Jan. 1994, pp. 10-15, Susumu Kuwabata, et al., "Electrochemical Synthesis of Composite Films of Manganese Dioxide and Polypyrrole and Their Properties as an Active Material in Lithium Secondary Batteries".
Journal of Power Sources, vol. 25, No. 3, Mar. 1989, pp. 177-185, N. Ilchev, et al., "The Lithium-Manganese Dioxide Cell II. Behavior of Manganese Dioxide in Nonaqueous Electrolyte".
Database WPI, Derwent Publications, AN-95-191409, JP-7-111153, Apr. 25, 1995.

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