Hydrocarbon conversion using large crystal zeolite catalyst

Chemistry of hydrocarbon compounds – Aromatic compound synthesis – By alkyl or aryl transfer between molecules – e.g.,...

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208109, 208114, 208118, 208121, 20811101, 20811115, 423702, 423709, 423711, C07C 522, C10G 4712, C10G 4700, C10G 1102

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061601918

ABSTRACT:
A process for converting hydrocarbons by contacting a hydrocarbon feedstream under hydrocarbon conversion conditions with a large crystal zeolite catalyst. The large crystal zeolite of the catalyst used in the hydrocarbon conversion process is made by heating an aqueous zeolite synthesis mixture under agitation to a temperature equal to or less than the effective nucleation temperature of the synthesis mixture. After this step, the aqueous synthesis mixture is heated in the absence of agitation to a temperature equal to or greater than the effective nucleation temperature of the aqueous zeolite synthesis mixture. The process finds particular application in hydrocarbon conversion processes where reduced non-selective acidity is important for reaction selectivity and/or the maintenance of catalyst activity, e.g., toluene disproportionation, dealkylation, alkylation, and transalkylation.

REFERENCES:
patent: 3503874 (1970-03-01), Michalko
patent: 4375458 (1983-03-01), Dwyer et al.
patent: 4650656 (1987-03-01), Dwyer et al.
Patent Abstracts of Japan, vol. 008, No. 114 (C-225), May 26, 1984 and JP 59026917A (KAO Sekken KK), Feb. 13, 1984.

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