Hydride compounds with silicon and germanium core atoms and...

Chemistry of inorganic compounds – Silicon or compound thereof

Reexamination Certificate

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C423S644000, C117S939000, C148SDIG058

Reexamination Certificate

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07981392

ABSTRACT:
A method is provided for synthesizing silicon-germanium hydride compounds of the formula (H3Ge)4-XSiHX, wherein x=0, 1, 2 or 3. The method includes combining a silane triflate with a compound having a GeH3ligand under conditions whereby the silicon-germanium hydride is formed. The compound having the GeH3ligand is selected from the group consisting of KGeH3, NaGeH3and MR3GeH3, wherein M is a Group IV element and R is an organic ligand. The silane triflate can be HXSi(OSO2CF3)4-xor HxSi(OSO2C4F9)4-x. The method can be used to synthesize trisilane, (H3Si)2SiH2, and the iso-tetrasilane analog, (H3Si)3SiH, by combining a silane triflate with a compound comprising a SiH3ligand under conditions whereby the silicon hydride is formed. The silane triflate can include HXSi(OSO2CF3)4-xor HXSi(OSO2C4F9)4-xwherein x=1 or 2. A method for synthesizing (H3Ge)2SiH2includes combining H3GeSiH2(OSO2CF3) with KGeH3under conditions whereby (H3Ge)2SiH2is formed.

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Supplemental ISR EP 05746524, mailed Jan. 31, 2011.

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