High molecular weight polystannanes by metal-catalyzed dehydropo

Synthetic resins or natural rubbers -- part of the class 520 ser – Synthetic resins – From heavy metal or aluminum reactant having at least one...

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528395, 556 11, 556 12, 556 28, 556 82, C08G 7900

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054880912

ABSTRACT:
A method for coupling tin-containing molecules via a Sn--Sn bond is described. The invention employs dehydrocondensation to link the Sn atoms of two molecules to form tin dimers as well as novel high molecular weight organotin polymers. In a preferred embodiment, catenated tin polymers are formed from hydrostannane precursors in the presence of a suitable metal catalyst. A particularly preferred method involves coupling dialkylstannane monomers in the presence of a metallocene catalyst to form polystannanes. Preferred catalysts include electropositive metals, such as Zr and Hf. The polystannanes are photolabile, decomposing readily under room light conditions.

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Sita, L. R. "A New Strategy for the Synthesis of Homologously Pure Linear Polystannane . . . " Organomet. 11:1442 (1992).

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