Enzymatic process to separate racemic mixtures of delta valerola

Organic compounds -- part of the class 532-570 series – Organic compounds – Heterocyclic carbon compounds containing a hetero ring...

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549292, 549328, C07D30430, C07D30512

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active

054121108

ABSTRACT:
Process to separate racemic mixtures of beta-hydroxy or beta-acyloxy-delta-valerolactones, which in position 2 and/or 5 of the lactone ring are substituted by hydrogen, alkyl groups having 4 to 20 C atoms, which are optionally penetrated by an oxygen atom, or by aralkyl groups, whereby not both positions are substituted by hydrogen, through reaction of the racemic mixture in the presence of a hydrolase with or without esterifying agent in a diluent and separation of the reaction mixture, which contains an enantiomerically pure beta-hydroxy-delta-valerolactone and an enantiomerically pure beta-acyloxy-delta-valerolactone, through conventional methods into the enantiomically pure compounds,
a process for the manufacture of enantiomerically pure oxetanones using said separation process and enantiomerically pure beta-acyloxy-delta-valerolactones.

REFERENCES:
patent: 4963492 (1990-10-01), Keller et al.
patent: 5084392 (1992-01-01), Miyazawa et al.
Laymen et al, J. Chem. Soc., Chem. Commun. (1988), pp. 1459-1461.

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