Derivatization of amines for electrochemical detection

Chemistry: analytical and immunological testing – Nitrogen containing – Amine and quaternary ammonium

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436106, 436112, 436161, 436816, 436901, G01N 3002, G01N 3064, G01N 3348

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active

049083228

ABSTRACT:
Primary and secondary amines in biological fluids are selectively derivitized by reaction with esters of N-hydroxysuccinimide or N-hydroxysulfosuccinimide to form an N-acylated derivative. Those N-acylated derivatives may then be extracted into a polar organic phase and extracted. Non-electroactive amines may be made suitable for coulometric analysis by selecting the ester used so as to attach an electroactive group to the amine. For example, histamine may be reacted with the Bolton-Hunter reagent to form a suitable derivative in high yield.

REFERENCES:
patent: 4288547 (1981-09-01), Yamamoto
patent: 4412068 (1983-10-01), Rosi
patent: 4430263 (1984-02-01), March et al.
"Microdetermination of Hydrazine Salts & Certain Derivatives w/N-Chlorosuccinimide," Anal. Chem., 46(6), pp. 777-779.
"Simultaneous Determination of Histamine and N.sup..tau. -Methylhistamine With High-Performance Liquid Chromatography Using Electrochemical Detection," Analytical Biochemistry, I52, pp. 127-135.
CA 91:222032e, New Derivatization of Amines for Electrochemical Detection in Liquid Chromatography.

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