Cyclic process for oxidation of calcium sulfide

Catalyst – solid sorbent – or support therefor: product or process – Regenerating or rehabilitating catalyst or sorbent – Gas or vapor treating

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502 38, 502 49, 502 51, 502 52, 423638, B01J 2034, C01B 1314

Patent

active

060838620

ABSTRACT:
Calcium sulfide particles in mixtures with carbon particles, as in coal gasifier waste, are converted to calcium oxide by repeated cycles of oxidation and reduction by utilizing the carbon as a source of the reducing gas required for the treatment. The treatment can be conducted in a two zone fluidized bed reactor by limiting the amount and concentration of oxygen supplied to a lower reducing zone and by supplying excess oxygen to an upper oxidizing zone. Alternatively, for particles less than 0.5 mm in size, the treatment can be conducted by utilizing either two transport reactors or two circulating fluidized bed reactors in series whereby the first reactor in the series is maintained in a reducing state and the second reactor is maintained in an oxidizing state. The particles are transported sequentially through both reactors and recycled several times. The amount and concentration of oxygen supplied to the first reactor is limited to create reducing conditions, while excess oxygen is supplied to the second reactor to create oxidizing conditions.

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