Crystalline microporous metal sulfide compositions

Catalyst – solid sorbent – or support therefor: product or process – Catalyst or precursor therefor – Selenium or tellurium or compound containing same

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502216, 502219, 502220, 502222, 423508, 423509, 4235611, 4235661, B01J 2704, C01B 1720

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048807613

ABSTRACT:
This invention relates to a crystalline composition having a three-dimensional microporous structure of MA.sub.2 units where A is sulfur or selenium and having the empirical formula expressed in molar ratios: xR:MA.sub.2.+-.0.2 :zH.sub.2 O where R represents at least one organic templating agent present in the intracrystalline pore system, x is the moles of R, z is the moles of water and M is germanium or tin. This invention also relates to a composition having the empirical formula expressed in molar ratios: xR:M.sub.1-y M'.sub.y A.sub.2.+-.0.2 :zH.sub.2 O, where M' is a metal such as cobalt, zinc, manganese, iron, nickel, copper, cadmium and gallium. This invention further relates to a method of preparing the crystalline composition.

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B. Krebs, "Thio- and Seleno-Compounds of Main Group Elements--Novel Inorganic Oligomers and Polymers", Angew. Chem. Int. Ed. Engl. 22 (1983) 113-134.
M. Evain, M. Queignec and R. Brec and C. Sourisseau, "Chalcogen Substitution in the Ta.sub.4 P.sub.4 S.sub.29 Tunnel Structure: Synthesis and Structure of TaPS.sub.6 Se", vol. 75, 413-431 (1988).

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