Chromatographic separation of zirconium isotopes with anhydrous

Chemistry of inorganic compounds – Treating mixture to obtain metal containing compound – Group ivb metal

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423 2, 423 69, 423 73, B01D 1508, C22B 3414, C10G 2500, C10G 2700

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050230611

ABSTRACT:
The isotopes of zirconium can be partially or completely separated by loading an essentially anhydrous alcoholic solution of an ionic compound of zirconium onto a cationic exchange resin with pentavalent phosphorus derived active groups which serves as the stationary phase of a chromatograph, eluting the compound with an essentially anhydrous alcoholic solution of hydrogen chloride and collecting distinct elution volumes representative of each isotope. In a preferred embodiment, the active groups of the cation exchange resin are derived from di-2-ethylhexyl phosphoric acid, tri-n-octyl phosphine oxide or tributyl phosphate and the chromatograph is of a type, such as a continuous annular chromatograph that it can be operated in a continuous steady state manner.

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Byers et al., "Pilot-Scale Studies of Sugar Separations by Continuous Chromatography", Oak Ridge National Laboratory, pp. 1-29.

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