Chain transfer reagent, free radical polymerization...

Synthetic resins or natural rubbers -- part of the class 520 ser – Synthetic resins – Polymers from only ethylenic monomers or processes of...

Reexamination Certificate

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C526S117000, C526S170000, C526S171000, C526S172000, C526S303100, C526S305000, C526S307100, C526S307800, C526S317100, C526S346000, C525S384000, C556S015000, C556S016000

Reexamination Certificate

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07132491

ABSTRACT:
Organometallic reversible addition-fragmentation chain transfer reagents (RAFT reagents), processes of free radical polymerization employing the same and polymers with low polydispersity index obtained thereby. The process includes polymerizing at least one monomer with at least one initiator and at least one organometallic RAFT reagent to obtain polymers having terminal organometallic functional groups with low polydispersity index. In addition, the terminal organometallic functional group may be removed by subjecting the obtained polymer to elimination to provide the corresponding organic polymers.

REFERENCES:
patent: 6667376 (2003-12-01), Charmot et al.
Mayadunne et al, Living Radical Polymerization with Reversible Addition-Fragmentation Chain Transfer . . . Using Dithiocarbamates as Chain Transfer Agents, Macromolecules, 1999, 32, 6977-6980.
Yih et al, Syntheses, Reactivities and Molecular Structures of Tungsten Complexes containing the Diphenylphosphinodithioformato Ligand, J. Chem. Soc. Dalton Trans. 1995, 1305-1313.
Yih and Lin, Syntheses and reactivity of molybdenum complexes containing the diphenylphosphinodithioformato ligand, Journal of Organometallic Chemistry 577 (1999) 134-139.

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