Catalytic oxidation of solid materials

Metal treatment – Compositions – Heat treating

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29571, 29590, 357 5, 427331, 4274193, 148DIG16, 148DIG89, 148DIG117, 148DIG118, H01L 21363

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045266298

ABSTRACT:
One or more monolayers of cerium arrayed on the surface of a niobium metal acts as a catalyst to oxidation of the niobium at ambient temperature and results in a very thin, very high quality insulating layer which may be configured by patterning of the catalyst. Significant amounts of Nb.sub.2 O.sub.5 are formed at pressures as low as 6.6.times.10.sup.-6 Pa, promoted by the presence of the cerium. This catalytic activity is related to the trivalent to tetravalent valence change of the cerium during oxidation. The kinetics of Nb.sub.2 O.sub.5 formation beneath the oxidized cerium shows two stages:

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Matsuda et al.; Study of Nb-Based Josephson Tunnel Junctions, J. Appl. Phys., vol. 51, No. 8, pp. 4310-4316, Aug. 1980.
Broom et al.; Niobium Oxide-Barrier Tunnel Junction, IEEE Trans. Elec. Dev., vol. ED-27, No. 10, pp. 1998-2008, Oct. 1980.

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