Catalysts for photo-assisted oxidation-reduction reactions

Chemistry: electrical and wave energy – Processes and products – Processes of treating materials by wave energy

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20415749, 2041575, 20415752, 204903, 502208, 502210, 502216, 501134, 501136, B01J 1912, B01J 2714, B01J 27188, B01J 2702

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046234373

ABSTRACT:
New catalysts for photo-assisted (i.e. promoted by light) oxidation-reduction (redox) reactions are disclosed. These catalysts consist of colloidal particles of a semiconductor, containing on their surface a reduction catalyst and an oxidation catalyst. In a first class of catalysts, the semiconductor has a difference of energy between valence band and conduction band such as to allow the hole-electron separation by absorption of visible light. This semiconductor is selected, in the case of the photo-decomposition of water, from the group consisting of TiO.sub.2 doped with Mn, Cr, or Cr and Nb; CdS doped with In or Ga; SrTiO.sub.3 doped with Cr or Mn; gallium phosphide; and cadmium sulphoselenide. In the case of the other photo-decomposition reactions, the semiconductor is selected from the group consisting of the above-mentioned compounds and CdS.
In a second class of catalysts, the semiconductor has a difference of energy between valence band and conduction band such as not to permit the hole-electron separation by absorption of visible light. This semiconductor is selected, in the case of the photo-decomposition of water, from the group consisting of SrTiO.sub.3 and Nb.sub.2 O.sub.5. In the case of the other photo-decompositon reactions, the semiconductor is selected from the group consisting of the above-mentioned compounds and TiO.sub.2 doped with Nb.

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