Catalysts for oxidative steam reforming of methanol as a new...

Chemistry of inorganic compounds – Hydrogen or compound thereof – Elemental hydrogen

Reexamination Certificate

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C502S346000

Reexamination Certificate

active

07025947

ABSTRACT:
The present invention provides a method of producing a CuZnAlZr oxide catalyst consisting of reacting an aqueous NaOH solution and aqueous Na2CO3solution with a mixture of aqueous solutions of each nitrate of Cu, Zn, Al, and Zr, producing a precipitate by coprecipitation, aging, filtering, washing and drying this precipitate to prepare a catalyst precursor consisting of a CuZnAlZr layered double hydroxide, and then obtaining a CuZnAlZr oxide by calcining this precursor in an air ambient atmosphere, a CuZnAlZr oxide catalyst, a CuZnZrCe oxide catalyst, a CoCuZnAl oxide catalyst for producing hydrogen by oxidative steam reforming a methanol, and methods of producing hydrogen gas consisting of converting methanol to hydrogen gas by oxidative steam reforming in the presence of air and steam using these oxide catalysts.

REFERENCES:
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patent: 6576217 (2003-06-01), Nojima et al.
S. Velu, et al., “Oxidative Steam Reforming of Methanol Over CuZNAI(Zr)-Oxide Catalysts: A New and Efficient Method for The Production of Co-Free Hydrogen For Fuel Cells,” Chem. Communications, No. 23, Dec. 7, 1999, pp. 2341-2342.
S. Velu, et al., “Oxidative Steam Reforming of Methanol Over CuZnAI(ZR)-Oxide Catausts for the Selective Production of Hydrogen for Fuel Cells: Catalyst Characterization and Performance Evaluation,” Journal of Catalyst, 194, 2000, pp. 373-384.
S. Velu, et al., “A Comparative Study of Reactions of Methanol Over Catalysts Derived From NiAI-and CoAO-Layered Double Hydroxidesa and Their Sn-Containing Analogues,” Catalysis Letters, 69, 2000, pp. 43-50.
John P. Breen, et al., Methanol Reforming for Fuel-Cell Applications: Development of Zirconia-Containing Cu-Zn-Al Cataysts,: Catalysis Today, 51, 1999, pp. 521-533.
J. L. G. Fierro, “Oxidative Methanol Reforming Reactions for the Production of Hydrogen,” Studies in Surface Science and Catalysis, 130, 2000, pp. 177-186.
Alakananda Bhattacharyya, (WO9903779 A1, Jan. 28, 1999), “Preparation and Calcination of Hydrotalcite-Type Compounds as Steam Reforming Catalysts for Oxygen-Containing Feedstocks,” Americal Chemical Socitey (Abstract Only).

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