Catalyst system for treating the exhaust from a lean-burn gasoli

Catalyst – solid sorbent – or support therefor: product or process – Zeolite or clay – including gallium analogs – And additional al or si containing component

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4232135, B01J 2930

Patent

active

051853051

ABSTRACT:
A catalyst system for converting NO.sub.x, CO, and HC contained in the exhaust gas from a gasoline-fueled engine controlled to operate under lean-burn conditions (R=0.03-0.9) such that the a ratio of NO.sub.x to HC in the exhaust gas in in the range of 1/3 to 3/1 (i.e., minimum C.sub.3 H.sub.6 of 250 ppm and NO.sub.x of 200-400 ppm). The system comprises a first stage catalyst containing a transition metal-exchanged zeolite (i.e., Cu-ZSM5), and a three-way catalyst for treating the effluent from said first stage catalyst. The second stage catalyst consists of a high surface area alumina support impregnated with an intimate mixture of 0.5-20% lanthana, 0.2-30% palladium, and advantageously an outer washcoat TiO.sub.2.
A method of treating the exhaust gas from a fossil-fueled engine comprising operating the engine under lean-burn conditions while controlling the emission ratio of NO.sub.x /hydrocarbon to be in the range of 1/3 to 3/1; exposing the exhaust gas to a first stage catalyst comprising a copper ion-exchanged ZSM5 zeolite having at least 3% by weight copper; and exposing the effluent from said first stage catalyst to a second stage catalyst comprising an alumina support impregnated with an intimate mixture of 0.5-20% lanthana and 2-30% palladium.

REFERENCES:
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patent: 5021389 (1991-06-01), Chatta et al.
patent: 5051244 (1991-09-01), Dunne et al.
patent: 5063192 (1991-11-01), Murakami et al.
"Automobile Catalytic Converters", Taylor, Springer, Berlin 1984, p. 107.
"Cu-ZSM-5 Zeolite as Highly Active Catalyst for Removal of Nitrogen Monoxide from Emission of Diesel Engines", Sato et al., Applied Catalysis, vol. 70, L1-15, 1991.

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