Bis(silyl)alkanes and method for their preparation

Organic compounds -- part of the class 532-570 series – Organic compounds – Silicon containing

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C07F 708

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052350835

ABSTRACT:
Bis(silyl)alkanes represented by the formulas (III), (IV) and (V) ##STR1## wherein R is H or phenyl, R' is a hydrogen atom or C.sub.1-4 alkyl and n is an integer ranging from 1 to 4. The present invention also provides a method for preparation of the bis(silyl)alkanes comprising the steps of mixing an organic compound, which is represented by the formula (I) and has a chloro at each side of its molecule, with a hydrogen chloride or an organic chloride represented by the formula (II), the organic chloride being capable of generating the hydrogen chloride during its reaction, in order to provide a mixture and directly reacting this mixture with a metal silicon at a reaction temperature of 260.degree. C.-370.degree. C. in the presence of a copper catalyst.

REFERENCES:
patent: 5075477 (1991-12-01), Jung et al.
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"Catalyst Based on Copper Used in the Synthesis of the Methylchlorosilanes" by P. Trambouze et al., J. Chim. Phys., 51, 505 (1954).
"Mechanism and Kinetics of the Metal-Catalyzed Synthesis of Methylchlorosolanes. III. The Catalytically Active Form of the Copper Catalyst" by R. J. H. Voorhoeve et al., J. Catalysis, 4, 123 (1965).
"Organohalosilanes: Precursors to Silicones" by J. C. Vlugter et al., Conf. Accad. Lincei: Alta. Tech. Chim., 1961, p. 81 (1962).
"Formation of Organosilicon Compounds. 102." by G. Fritz et al., Z. Anorg. Allg. Chem., 512, 131 (1984).
"Synthesis of Organosilicon Compounds. XI. Formation of Silicon Methylene Compounds from Dichloromethane and Silicon", Z. Anorg. U. Allgem. Chem., 306, 39 (1960).

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