Drug – bio-affecting and body treating compositions – Designated organic active ingredient containing – Having -c- – wherein x is chalcogen – bonded directly to...
Reexamination Certificate
2002-06-17
2004-01-20
Pryor, Alton N (Department: 1616)
Drug, bio-affecting and body treating compositions
Designated organic active ingredient containing
Having -c-, wherein x is chalcogen, bonded directly to...
C514S256000, C514S365000
Reexamination Certificate
active
06680325
ABSTRACT:
FIELD OF THE INVENTION
The present invention relates to pesticides which comprise an active compound combination of the compound of the formula (I)
with fungicides.
BACKGROUND OF THE INVENTION
Fungicidally active compounds, such as azole derivatives, aryl benzyl ethers, benzamide, morpholine compounds and other heterocycles, are known (cf. K. H. Büchel “Pflanzenschutz und Schädlingsbekämpfung”, pages 140 to 153, Georg Thieme-Verlag, Stuttgart 1977, EP published specification 0 040 345, German Offenlegungsschrift 2 324 010, German Offenlegungsschrift 2 201 063, EP published specification 0 112 284, EP published specification 0 304 758 and DD patent specification 140 412).
Mixtures of certain nitromethylene derivatives with fungicidally active compounds and their use as pesticides in crop protection are already known (U.S. Pat. No. 4,731,385; JP published specifications 63-68507, 63/68505; 63172 608; 63/72 609, 63/72 610, WO 96/03 045, Japanese patent specification 08 245 323, Japanese patent specification 04 368 303, Japanese patent specification 05 017 311, WO 92/21 241, WO 97/22 254). Mixtures of certain open-chain nitromethylenes and nitroguanidines with fungicides are already known (Japanese published specification 30 47 106; U.S. Pat. No. 5,181,587).
Mixtures of cyclopropylcarboxamides with certain nitromethylene or nitroguanidine derivatives are already known (Japanese published specification 3 271 207).
Mixtures of, inter alia, imidacloprid and fungicidally active compounds for use in the protection of materials and against termites, but not for use against plant-damaging pests, are already known (EP published specification 0 511 541). Mixtures of imidacloprid and azolylmethylcycloalkanes, in particular triticonazole, are known from EP published specification 545 834.
DETAILED DESCRIPTION OF THE INVENTION
However, hitherto it has not been known that nitroguanidine derivatives and fungicides with the exception of cyclopropylcarboxamides and triticonazole have such a mutually beneficial effect in their activity that they are outstandingly suitable as compositions for controlling plant pests, whilst being tolerated well by plants.
The present invention relates to compositions against plant pests which contain the compound of the formula (I)
in a mixture with fungicidally active compounds, except for cyclopropylcarboxamide derivatives and azolylmethylcycloalkanes.
Examples of fungicides in the compositions according to the invention for controlling plant pests which may be mentioned are:
(1) Azole Derivatives of the Formula
The active compound of the formula (I) is known from EP published specification 0 375 907.
The fungicidal active compounds are also known.
Thus, for example, the following publications describe:
(1) Compounds of the Formula (II) DE published specification 2 201 063 DE published specification 2 324 010 DE published specification 2 737 489 DE published specification 3 018 866 DE published specification 2 551 560 EP 47 594 DE 2 735 872
(2) The Compound of the Formula (III) EP 68 813 U.S. Pat, No. 4,496,551
(3) The Compound of the Formula (IV) DE published specification 2 429 523 DE published specification 2 856 974 U.S. Pat. No. 4,108,411
(6) Compounds of the Formula (VII) DL 140 041
(7) The Compound of the Formula (VII) EP 382 375
(8) The Compound of the Formula (IX) EP 515 901
(9) The Compound of the Formula (X) EP 314 422
(10) The Compound of the Formula (XI) EP 49 854
(11) The Compound of the Formula (XII) DE published specification 1 770 288 U.S. Pat. No. 3,869,456
(13) Compounds of the Formula (XIV) DE 2 207 576 U.S. Pat. No. 3,903,090 U.S. Pat. No. 3,755,350 U.S. Pat. No. 3,823,240
(14) Compounds of the Formula (XV) EP270 111
(19) The Compound of the Formula (XX) EP 219 756
(34) The Compound of the Formula (XXXV) U.S. Pat. No. 4,512,989
(38) Compounds of the Formula (XXXIX) EP 398 692
(48) Compound From WO 97/27189
(49) Compound From WO 96/16048, this compound can be present in 2 tautomeric forms (A) and (B)
Compounds from the groups (15), (16), (17), (18), (23), (34), (25), (28), (31), (32), (33) and (38) to (47) are described, for example, in K. H. Büchel, “Pflanzenschutz und Schädlingsbekämpfung”, pages 121-153, Georg Thieme-Verlag, Stuttgart, 1977.
The compound of group (39) is known from EP published specification 281 842.
The compound of group (50) is known from WO 97/ 06 171.
The compound of group (51) is known from DE-24 33 410.
The compounds of groups (52) to (54) are known from W. Paulus, “Microbicides for the Protection of Materials”, Chapman & Hall 1993.
The compound of group (55) is known from EP-0 512 349.
In addition to the active compound of the formula (I), the active compound combinations according to the invention contain at least one fungicidal active compound, for example selected from the compounds of groups (1) to (55). In addition, they may also contain other active compounds and customary auxiliaries and additives and also diluents.
Preferred fungicidally active compounds in the compositions according to the invention are:
kresoxim-methyl, tebuconazole, metalaxyl, azoxystrobin, triadimenol, bitertanol, fenpicolonil, cyproconazole, propiconazole, fludioxonil and triazoxides.
The mixtures show a clear synergistic effect when the active compounds in the active compound combinations according to the invention are present in certain weight ratios. However, the weight ratios of the active compounds in the active compound combinations can be varied within a relatively wide range. In general,
0.1 to 10 parts by weight, preferably
0.3 to 3 parts by weight of at least one fungicidal active compound, for example from groups (1) to (55),
are present per part by weight of active compound of the formula (I).
The active compound combinations according to the invention have very good fungicidal properties. They can be employed in particular for controlling phytopathogenic fungi, such as Plasmodiophoromycetes, Oomycetes, Chytridiomycetes, Zygomycetes, Ascomycetes, Basidiomycetes, Deuteromycetes, etc.
The active compound combinations according to the invention are particularly suitable for controlling cereal diseases, such as Erysiphe, Cochliobolus, Septoria, Pyrenophora and Leptosphaeria, and against fungal attack on vegetables, grapevines and fruits, for example against Venturia or Podosphaera on apples, Uncinula on grapevines or Sphaerotheca on cucumbers.
The active compound combinations are also highly suitable for controlling animal pests, preferably arthropods, in particular insects, which are encountered in agriculture, in forestry, in the protection of stored products and of materials, and in the hygiene sector. They are active against normally sensitive and resistant species and against all or some stages of development. The abovementioned pests include:
From the order of the Isopoda, for example,
Oniscus asellus, Armadillidium vulgare
and
Porcellio scaber.
From the order of the Diplopoda, for example,
Blaniulus guttulatus.
From the order of the Chilopoda, for example,
Geophilus carpophagus
and Scutigera spec.
From the order of the Symphyla, for example,
Scutigerella immaculata.
From the order of the Thysanura, for example,
Lepisma saccharina.
From the order of the Collembola, for example,
Onychiurus armatus.
From the order of the Orthoptera, for example,
Blatta orientalis, Periplaneta americana, Leucophaea maderae, Blattella germanica, Acheta domesticus
, Gryllotalpa spp.,
Locusta migratoria migratorioides, Melanoplus differentialis
and
Schistocerca gregaria.
From the order of the Dermaptera, for example,
Forficula auricularia.
From the order of the Isoptera, for example, Reticulitermes spp.
From the order of the Anoplura, for example, Pediculus humanus corporis, Haematopinus spp. and Linognathus spp.
From the order of the Mallophaga, for example, Trichodectes spp. and Damalinea spp.
From the order of the Thysanoptera, for example,
Hercinothrips femoralis
and
Thrips tabaci.
From the order of the Heteroptera, for example, Eurygaster spp.,
Dysdercus intermedius, Piesma quadrata, Cimex lectularius, Rhodnius
Andersch Wolfram
Erdelen Christoph
Krämer Wolfgang
Mauler-Machnik Astrid
Stenzel Klaus
Bayer Aktiengesellschaft
Henderson Richard E. L.
Mrozinski, Jr. John E.
Pryor Alton N
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