Acylase gene

Chemistry: molecular biology and microbiology – Micro-organism – tissue cell culture or enzyme using process... – Preparing compound having a 1-thia-5-aza-bicyclo

Reexamination Certificate

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C435S230000, C435S320100, C435S252330, C435S069100, C435S252300, C536S023200, C536S023100, C536S023700, C536S024100

Reexamination Certificate

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10516587

ABSTRACT:
The subject of the present invention is to provide a β-lactam acylase protein having high activity, a gene coding for said β-lactam acylase protein, a recombinant vector having said gene, a transformant containing said recombinant vector, and a method of producing a β-lactam antibiotic such as amoxycillin using said β-lactam acylase. A β-lactam acylase gene ofStenotrophomonas maltophiliawas cloned, the DNA base sequence and the amino acid sequence expected therefrom was determined, and aStenotrophomonasβ-lactam acylase gene was obtained. This gene was found to code for a protein with a molecular weight of about 70 kDa and having β-lactam acylase activity, and could efficiently produce amoxycillin without being inhibited by phenylacetic acid, etc. Furthermore, by modification of the amino acid sequence, a protein which can more efficiently produce amoxycillin could be obtained.

REFERENCES:
patent: 5168048 (1992-12-01), Quax
patent: 4-228073 (1992-12-01), None
Crowder, Michael, W., et al., Overexpression, Purification, and Characterization of the Cloned Metallo-β-Lactamase L1 fromStenotrophomonas maltophilia, Antimicrobial Agents and Chemotherapy,vol. 42, No. 4, Apr. 1998, p. 921-926.
Hernández-Jústiz, O., et al., Evaluation of different enzymes as catalysts for the production of β-lactam antibiotics following a kinetically controlled strategy,Enzyme and Microbial TechnologyApr. 25, 1999, p. 336-343.
Simpson et al., “The genome sequence of the plant pathogenXylella fastidiosa,” Nature, vol. 408, pp. 151-157 (Jul. 13, 2000).
Kim et al., “Characterization of Glutaryl 7-ACA Acylase fromPseudomonas diminutaKAC-1,” J. Microbiology and Biotechnology (The Korean Society for Applied Microbiology), vol. 11, No. 3, pp. 452-457 (2001, Seoul, S. Korea).
Elander, “Industrial production of β-lactam antibiotics,” Applied Microbiology and Biotechnology, vol. 61, pp. 385-392 (2003).
Sio et al., “Improved β-lactam acylases and their use as industrial biocatalysts,” Current Opinion in Biotechnology, vol. 15, pp. 349-355 (2004).
Database UniProt (Online), Oct. 1, 2000, “Glutaryl-7-ACA Acylase”, Amino Acid Sequence, Accession No. Q9PEJ9, XP-002375572.

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