Poly (ethylene/alkylene) terephthalates which crystallize rapidl

Synthetic resins or natural rubbers -- part of the class 520 ser – Synthetic resins – From carboxylic acid or derivative thereof

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264176R, 264176F, 528298, 528302, 528305, 528307, C08G 6318

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active

041762240

ABSTRACT:
The present invention is concerned with thermoplastic terephthalic acid copolyesters which crystallize more rapidly than homopolyethylene terephthalate and are based on a diol component which is about 98 to 99.9 mol % of ethylene glycol and the balance 2-ethylhexane-1,3-diol. The acid component may be up to about 10.0 mol % of other than terephthalic acid or its dimethyl ester.
This invention is also concerned with a process of synthesizing such copolyesters by esterifying or transesterifying the acid and diol components between about 150.degree. and 250.degree. C. in the presence of appropriate catalysts. The condensation product may be subject to polycondensation at about 200.degree. to 300.degree. C. under reduced pressure in the presence of esterification catalysts. In a preferred embodiment the 2-ethylhexane-1,3-diol is added after the initial reaction between the acid component and the ethylene glycol and preferably after the degree of polycondensation is greater than 4.

REFERENCES:
patent: 3692744 (1972-09-01), Rich et al.
patent: 3934067 (1976-01-01), Goldman et al.
patent: 4086212 (1978-04-01), Bier et al.
Wilfong, J. Polym. Sci., 54, (1961), pp. 385-410.
Abraham et al., Chemical Abstracts, vol. 82:59,347q (1975).

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