Supported ionic catalyst composition

Catalyst – solid sorbent – or support therefor: product or process – Catalyst or precursor therefor – Plural component system comprising a - group i to iv metal...

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502120, 502152, 502155, 526160, 526901, 526943, 526352, 526351, 5263482, C08F 464

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active

056438478

ABSTRACT:
The invention is directed to a catalyst composition suitable for addition reactions of ethylenically and acetylenically unsaturated monomers comprising a metal oxide support having covalently bound to the surface thereof directly through the oxygen atom of the metal oxide an activator anion that is also ionically bound to a catalytically active transition metal cation compound. The invention includes a preparation process for the invention catalyst composition exemplified by reacting a Lewis acid, such as trisperflourophenyl boron with residual silanol groups of a silica support, preferably then reacting with a Lewis base such as diethylaniline, so as to prepare a silica bound anionic activator that when combined with a suitable transition metal compound will protonate it so as to form the ionic catalyst system. Use of the invention catalyst to polymerize alpha-olefins is exemplified.

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"Olefin Copolymerization with Metallocene Catalysts. III Supported Metallocene/Methylaluminoxane Catalyst for Olefin Copolymerization" pp. 1603-1607: J. Polym. Sci., A, Polym Chem, vol. 29,1991.
Yang et al. "Cation-like" Homogeneous Olefin Polymerization Catalysts Based upon Zirconocene alkyls and Tris(pentafluorophenyl)borane, J. Am. Chem. Soc. 1991,113, pp. 3623-3625 1991.
Quyoum et al. ".eta.-C5TiMe3B(C6F5)3: A Carbocationic Olefin Polymerization Initiator Masquerading as a Ziegler-Natta Catalyst" J. Am. Chem. Soc. 1994, 116, 6435-6436.
M.P. McDaniel "Supported Chromium Catalysts for Ethylene Polymerization" Advances in Catalysis, vol. 33, pp. 47-97 (1985).

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