Separation of pure optical stereoisomers by pressure crystalliza

Organic compounds -- part of the class 532-570 series – Organic compounds – Oxygen containing

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568810, 568831, 568832, 568833, C07C 3512, C07C 2978

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active

050196588

ABSTRACT:
The instant invention is an improvement in the method of producing optically pure sterioisomers from a racemic mixture. The method is based on the well-known fact that a supersaturated solution or melt of the racemic mixture can be seeded with just the crystals of the desired stereoisomer, which will then crystallize out selectively, leaving the undesired stereoisomer behind in the liquid mother liquor. The desired isomer, in crystaline form, can then be separated by simple liquid/solid separation from the undesired isomer remaining behind in the mother liquor. In the conventional method, supersaturation is achieved by careful cooling of a saturated solution or melt. In the present invention, supersaturation is achieved by increasing the ambient pressure over the saturated solution or melt of the racemic mixture, and relying on the fact that the melting temperature of a substance increases with increasing pressure, provided there is an increase in molar volume when the substance melts.

REFERENCES:
patent: 3053880 (1962-09-01), Dale
patent: 3943181 (1976-03-01), Fleisher et al.
patent: 4011270 (1977-03-01), Carrington
patent: 4418225 (1983-11-01), House

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