Process of forming polysubstituted fullerenes

Organic compounds -- part of the class 532-570 series – Organic compounds – Carboxylic acid esters

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560 89, 564308, 568719, C07C 69753

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active

051772485

ABSTRACT:
The present invention is directed toward the preparation of novel polysubstituted fullerenes. The method of forming polysubstituted fullerenes comprises contacting a fullerene with an electrophilic reagent selected from the group consisting of nitronium ion and organic peracid, provided that when the electrophilic reagent is nitronium ion, the fullerene is subsequently contacted with a nucleophilic reagent.

REFERENCES:
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Joel M. Hawkins, et al., Organic Chemistry of C.sub.60 (Buckminsterfullerene): Chromatography and Osmylation, 1990, 55, 6250-6252, J. Org. Chem.
Stephen G. Kukolich, et al., EPR Spectra of C.sub.60 Anion and Cation Radicals, Aug. 2, 1991, vol. 182, No. 3.4, pp. 263-265, Chemical Physics Letters.
Paul J. Fagan, et al., The Chemical Nature of Buckminsterfullerene (C.sub.60) and the Characterization of a Platinum Derivative, May 24, 1991, vol. 252, pp. 1160-1161, Science.
George A. Olah, et al., Chlorination and Bromination of Fullerenes. Nucleophilic Methoxylation of Polychlorofullerenes and Their Aluminum Trichloride Catalyzed Friedel-Crafts Reaction with Aromatics to Polyarylfullerenes, 1991, 113, 9384-9387, J. Am. Chem. Soc.
George A. Olah, et al., Polyarenefullerenes, C.sub.60 (H-Ar).sub.n Obtained by Acid-Catalyzed Fullerenation of Aromatics, 1991, 113, 9387-9388, J. Am. Chem. Soc.

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