Method for extracting lanthanides and actinides from acid soluti

Chemistry of inorganic compounds – Treating mixture to obtain metal containing compound – Radioactive metal

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423 10, 423 215, B01D 1104, C01F 1700, C22B 5900, C01G 5600

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045740720

ABSTRACT:
A process for the recovery of actinide and lanthanide values from aqueous solutions with an extraction solution containing an organic extractant having the formula: ##STR1## where .phi. is phenyl, R.sup.1 is a straight or branched alkyl or alkoxyalkyl containing from 6 to 12 carbon atoms and R.sup.2 is an alkyl containing from 3 to 6 carbon atoms and phase modifiers in a water-immiscible hydrocarbon diluent. The addition of the extractant to the Purex process extractant, tri-n-butylphosphate in normal paraffin hydrocarbon diluent, will permit the extraction of multivalent lanthanide and actinide values from 0.1 to 12.0 molar acid solutions.

REFERENCES:
patent: 3243254 (1966-03-01), Siddall
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Navratil, J. D. and Martella, L. L. "Extraction Behavior of Americium and Plutonium with Mixed Solvent Extractants." Sep. Sci. and Tech., 16(9), pp. 1147-1155, 1981.
Horwitz et al., "The Extraction of Th(IV) and U(VI) by Dihexyl-N,N-diethylcarbamylmethylphosphonate from Aqueous Nitrate Media," pp. 403-416, Separation Science and Technology 16(4), (1981).
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Kalina et al., "The Extraction of Am(III) and Fe(III) by Selected Dihexyl-N,N-Dialkylcarbamoylmethyl-Phosphonates, -Phosphinates and -Phosphine Oxides from Nitrate Media," Separation Science & Tech., 16(9), pp. 1127-1145 (1981).
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Horwitz et al., "Carbamoylmethylphosphoryl Derivatives as Actinide Extractants and Their Significance in the Processing and Recovery of Plutonium and other Actinides," Plutonium Chemistry, ACS Symposium _Series, 216, Chapt. 22, p. 433 (1983).
Horwitz et al., "Octyl(Phenyl)-N,N-Diisobutylcarbamoylmethylphosphine Oxide as an Extractant for Actinides from Nitric Acid Waste," (ISEC '83).
Muscatello et al., "The Extraction of Americium(III) by Mixtures of Tributylphosphate with Dibutyl-N,N-diethylcarbamoylphosphonate and -Methylphosphonate (DBDECP and DBDECMP), "Solvent Extraction & Ion Exchange, 1(1) pp. 127-139 (1983).

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