Process for the preparation of isomelamines

Organic compounds -- part of the class 532-570 series – Organic compounds – Four or more ring nitrogens in the bicyclo ring system

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Other Related Categories

544197, C07D25170

Type

Patent

Status

active

Patent number

044992688

Description

ABSTRACT:
A novel process for the preparation of isomelamines of the formula I, ##STR1## which is characterized in that an N-cyano-N-(ar or cyclo)alkylcarboxylic acid amide or N-cyano-N-allylcarboxylic acid amide of the formula II or III ##STR2## is reacted with aqueous sodium hydroxide solution, potassium hydroxide solution or ammonia solution or a primary aliphatic or cycloaliphatic amine in a solvent or with a primary aliphatic alcohol in the presence of a catalytic amount of a basic compound in a temperature range from -20.degree. C. to 200.degree. C., at least 3 hydroxyl or amino group equivalents being used per 3 carboxylic acid amide group equivalents.
The isomelamines prepared by the process according to the invention are valuable curing agents for epoxide resins.

REFERENCES:
patent: 2481758 (1949-09-01), Kaiser et al.
patent: 2482076 (1949-09-01), Thurston
patent: 2485983 (1949-10-01), Nagy
patent: 2498217 (1950-02-01), Nagy et al.
patent: 3627734 (1971-12-01), Ohuchi et al.
S. A. Miller et al., J. Appl. Chem. 6, 89 (1956).
R. Kitawaki et al., J. Org. Chem. 25, 1043 (1960).
G. Rapi et al., J. Chem. Soc. (C), 1971, 3827.

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