Liquid chromatography/Fourier transform IR spectrometry interfac

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250341, 356246, 356440, G01J 100, G01N 110

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active

046187693

ABSTRACT:
A zero dead volume (ZDV) microbore high performance liquid chromatography (.mu.HPLC)/Fourier transform infrared (FTIR) interface flow cell includes an IR transparent crystal having a small diameter bore therein through which a sample liquid is passed. The interface flow cell further includes a metal holder in combination with a pair of inner, compressible seals for directly coupling the thus configured spectrometric flow cell to the outlet of a .mu.HPLC column end fitting to minimize the transfer volume of the effluents exiting the .mu.HPLC column which exhibit excellent flow characteristics due to the essentially unencumbered, open-flow design. The IR beam passes transverse to the sample flow through the circular bore within the IR transparent crystal, which is preferably comprised of potassium bromide (KBr) or calcium fluoride (CaF.sub.2), so as to minimize interference patterns and vignetting encountered in conventional parallel-plate IR cells. The long IR beam pathlength and lensing effect of the circular cross-section of the sample volume in combination with the refractive index differences between the solvent and the transparent crystal serve to focus the IR beam in enhancing sample detection sensitivity by an order of magnitude.

REFERENCES:
patent: 3985441 (1976-10-01), Schoeffel et al.
patent: 4009964 (1977-03-01), Bergen
patent: 4229179 (1980-10-01), Lee
patent: 4405235 (1983-09-01), Rossiter
Hirschfeld, "Dynamic Range Improvement in Fourier Transform Infrared Spectrometry", Anal. Chem. 50, 1978.
Brown et al., "Microbore Liquid Chromatography with Flow Cell Fourier Transform Infrared Spectrometric Detection", Anal. Chem. 55, 1983.
Johnson et al., "Zero Dead Volume Flow Cell for Microbore Liquid Chromatography with Fourier Transform Infrared Spec. Detection, Anal. Chem. 56, Dec. 1984.
Johnson et al., Tenth Quarterly Progress Report for Period, Jan. 1984--Mar. 1984, published Jun. 1984.

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